May I suggest a cap of your pavers on the wall and the a slightly darker gray that relates to the privacy fence beyond? That way horizontal surfaces and vertical surfaces show similarities and blends/blurs the separations?

As the appearance of the garden has a modernist style with the straight lines and concrete furniture how about a Mondrian influence and add a bold strip of blue? It is a pond and with the right shade it could look really relaxed and contemporary. My daughter's suggestion is a chalky lilac!

What a fun space! Love the pillows...I agree with above, lower all the frames, but not so low little ones can reach. The art should fall at eye level about 5'4" for walls and for behind the sofa not more than 12" above it. Then keep the width about 5" inside the sofa length on each side. Your frames are small so you need the close together for impact. I would start with some pretty curtains for the door and large window and then a simple Roman shade for the small window- since your girls play there you don't want anything they will grab hold of. http://www.houzz.com/ideabooks/query/how-to-hang-a-photo-gallery

I think the white trim gives it a much more contemporary look. It's more work to have it done in a different color, but the overall look is cleaner.